The U.S. Department of Energy’s Ames Laboratory has discovered and described the existence of a unique disordered electron spin state in a metal that may provide a unique pathway to finding and studying frustrated magnets.
Condensed matter physicists use the term “frustrated” to describe a kind of magnet in which the spins fail to align into stable magnetic order. In perfectly frustrated magnets called spin liquids, the disordered magnetism of these materials persists even at very low temperatures, and their unique properties are of interest in the development of quantum computing and high-temperature superconductivity.
The materials investigated to search for this perfectly frustrated magnetic state are typically insulators. But Ames Laboratory researchers were able to define a “perfectly frustrated” state in a metallic material, CaCo1.86As2.
“Perfectly frustrated systems, ones that really cannot resolve their magnetic states, are difficult to find in the first place, but even more so in a metal,” said Rob McQueeney, scientist at Ames Laboratory.
In insulating magnets, the interactions between spins that lead to frustration are set by the crystal structure of the lattice, and are relatively immutable. The discovery of this nearly perfectly frustrated metal provides a new avenue for tinkering with the magnetic interactions to achieve perfect frustration.
“Here, we have a little knob that we can tune. We know that some of these interactions that lead to frustration are mediated by conduction electrons, and we can tune a number of those very accurately—maybe you get a superconductor, maybe some other novel quantum state. There’s a lot of promise there.”
The research is further discussed in the paper Effective One-Dimensional Coupling in the Highly Frustrated Square-Lattice Itinerant Magnet CaCo2-yAs2, authored by A. Sapkota, B.G. Ueland, V.K. Anand, N.S. Sangeetha, D.L. Abernathy, M.B. Stone J.L. Niedziela, D.C. Johnston, A. Kreyssig, A.I. Goldman, and R.J. McQueeney; and published in Physical Review Letters.
This research used resources at the Spallation Neutron Source, a DOE Office of Science User Facility operated by Oak Ridge National Laboratory.
Ames Laboratory is a U.S. Department of Energy Office of Science national laboratory operated by Iowa State University. Ames Laboratory creates innovative materials, technologies and energy solutions. We use our expertise, unique capabilities and interdisciplinary collaborations to solve global problems.
DOE’s Office of Science is the single largest supporter of basic research in the physical sciences in the United States, and is working to address some of the most pressing challenges of our time. For more information, please visit science.energy.gov.
Robert McQueeney, Division of Materials Science and Engineering
Laura Millsaps, Ames Laboratory Public Affairs
A. Sapkota, B.G. Ueland, V.K. Anand, N.S. Sangeetha, D.L. Abernathy, M.B. Stone J.L. Niedziela, D.C. Johnston, A. Kreyssig, A.I. Goldman, and R.J. McQueeney
Effective One-Dimensional Coupling in the Highly Frustrated Square-Lattice Itinerant Magnet CaCo2-yAs2
Physical Review Letters 119, 147201 (2017)